Oxalic Acid Pretreatment, Fungal Enzymatic Saccharification and Fermentation of Maize Residues to Ethanol

Abstract
Dilute oxalic acid pretreatment was investigated as a feasible method for conversion of maize residues into sugars and subsequent production of bioethanol. Oxalic acid concentration of 200 mM for samples treated at 160°C for 10 min was found to be the best pretreatment conditions. Cellulases, mainly cellobiohydrolases from Trichoderma reesei, recorded activities of up to 116 U/ml during saccharification of the cellulosic substrates. The optimum saccharification conditions using 0.2% (v/v) enzyme concentrate were the incubation temperature of 45°C for 48 h. Up to 46% (w/w) glucose and 28% (w/w) xylose were obtained from the pretreated maize residues (stalk, leaf, husk and cobs). Furthermore, a native Saccharomyces cerevisiae (strain KB) was able to convert 78% (w/w) of glucose (and other fermentable sugars) to ethanol after 60 h of incubation at 32°C, under stationary culture conditions. The challenges encountered in chemical and biological conversions included incomplete hydrolysis and fermentation due to substrate recalcitrance and the inability of the yeast cells to utilize 5-carbon sugars such as xylose. This study therefore provided baseline research data and information that could be used for more elaborate and scaled-up studies for possible industrial-scale conversion of the readily available crop residues into bioenergy.
Description
Keywords
Bioethanol, cellulases, Cellulases, Fermentation, Hydrolysates, Maize residues, Oxalic acid, Pretreatment, Saccharification
Citation
Mtui, G.Y., 2012. Oxalic acid pretreatment, fungal enzymatic saccharification and fermentation of maize residues to ethanol. African Journal of Biotechnology, 11(4), pp.843-851.